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Best overland route from Lima to Tucuman, Argentina?

I want to travel overland by bus from Lima, Peru to Tucuman, Argentina through Chile or Bolivia, and need advice on the best travel route. The trip should span 6 weeks, so I can see some things, and not be exhausted by long bus rides. I will consider train segments, if they are popular, efficient and affordable. I will be staying at hostels along the way, and would appreciated advice on these also.

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